- Sean Connery - Dr. No - Dr. Julius No
- Sean Connery - From Russia with Love - Rosa Klebb
- Sean Connery - Goldfinger - Auric Goldfinger
- Sean Connery - Thunderball - Emilio Largo
- Sean Connery - You Only Live Twice - Blofeld
- George Lazenby - On Her Majesty's Secret Service - Blofeld
- Sean Connery - Diamonds Are Forever - Blofeld
- Roger Moore - Live and Let Die - Dr. Kananga
- Roger Moore - The Man with the Golden Gun - Francisco Scaramanga
- Roger Moore - The Spy Who Loved Me - Karl Stromberg
- Roger Moore - Moonraker - Sir Hugo Drax
- Roger Moore - For Your Eyes Only - Aristotle Kristatos
- Roger Moore - Octopussy - Kamal Khan
- Roger Moore - A View to a Kill - Max Zorin
- Timothy Dalton - The Living Daylights - Brad Whitaker with General Georgi Koskov
- Timothy Dalton - Licence to Kill - Franz Sanchez
- Pierce Brosnan - GoldenEye - Alec Trevelyan
- Pierce Brosnan - Tomorrow Never Dies - Elliot Carver
- Pierce Brosnan - The World Is Not Enough - Renard
- Pierce Brosnan - Die Another Day - Tan-Sun Moon
- Daniel Craig - Casino Royale - Mr. White with Le Chiffre & Alex Dimitrios
- Daniel Craig - Quantum of Solace - Dominic Greene
- Daniel Craig - Bond 23 - ???
